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Okay, I have three songs that I downloaded after suggestions from here. And I can't find what episodes they are actually in.
1. Hard to Live in the City - Albert Hammond Jr.
2. Oh My God - Ida Maria
3. We Started Nothing - The Ting Tings
If you have any idea, let me know.
Oh and this can be the sort of official forum where people can ask where a song was that they heard, or what song that they heard in some episode.
Number 1 is in the pilot when Chuck, Blair, Nate, Kati and Iz are in the limo.
2 I just remember it from the promos for eps 2.18-2.20
3 no clue