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I think they are Stefan and Katherine...
As much as I hate Jenny, I don't think she had planned to sleep with Chuck. And as much as I love Chuck, he was the one who made the first move. They both felt sad, lonely and miserable. He had nothing to struggle for (he thought he had lost Blair forever) and she was feeling hated by everyone. It was a mistake (of course!!!) but it happened on the spur of the moment, it wasn't planned.
I hope so. Both of them are great actors and we can feel their chemistry together. I would love to see them engaged by the end of the season, even if they break up and make up again, as always.