It doesn't look like Cas want's to go willingly with Bartholomew, but he's captured by him on "Captives."

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Diyah Pera/The CW
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Supernatural
Episode:
Supernatural Season 9 Episode 14: "Captives"
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Supernatural Season 9 Episode 14 Quotes

This is not happening. I spend months getting through the veil to listen to Dean Winchester having some pity session. I heard enough of those when I was alive.

Kevin

That's your third unanswered voicemail. Did you ever think maybe he's not that into you?

Sam