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Carina (Mini Anden) is back and is on a mission to steal a weapon from her fiance, Karl (Vinne Jones). Operation Chuck helps.
Chuck gets trained to become a real spy; Sarah and Casey go on a mission without him.
Chuck is determined to get Sarah back and when a CIA mission comes up where he gets to pick his choice of agent, he chooses Walker.
Chuck pretends to be an assassin, Rafe Gruber, hired by the mafia (Tony Sirico and Louis Lombardi) to kill Shaw.
Chuck and Sarah join Shaw on a mission to catch the Ring director that had Sarah kill his wife.
Shaw is back and convinces the CIA that Chuck and the Intersect are a danger.
When Chuck has problems flashing, he's left behind during a mission. With Sarah, Casey and Shaw gone, The Ring invades Castle.
Chuck and Sarah pose as a married couple on their honeyoon as they attempt to go AWOL from their spy lives together.
Chuck is given a final exam that if he passes will make him a full-fledged spy; Casey adjusts to civilian life.
Chuck must help Shaw steal the Mask of Alexander; Ellie and Morgan follow Chuck to figure out his secret.
Chuck is sent on his first solo mission to Paris this week. The episode is titled "Chuck Versus First Class."
Chuck begins having nightmares when the Intersect starts messing with his head and the CIA has him committed with guest start Christopher Lloyd as his psychiatrist.
Chuck and Sarah go on a mission to see if Shaw is still alive; Ellie manages to get Stephen Bartowski to return!
Casey is put on a side mission by his former boss gone Ring operative, James Kellar (Robert Patrick) and Casey and Sarah end up helping him commit treason.
After Devon saves the life of a Costa Grava dictator, he ends up involves in a spy mission with Chuck, Sarah and Casey.
Chuck and Sarah must train with the best spy couple ever, the Turners (Fred Willard and Swoosie Kurtz); Casey must train Morgan.
Chuck attempts to secure an asset working for the ring, Manoosh (Fahim Anwar); Morgan attempts to seduce Hannah (Kristin Kreuk).
Captain Awesome is kidnapped by Sydney (Angie Harmon) and is forced to shoot Shaw (Brandon Routh).